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For best ride quality you would run them a bit on the low side.
That said, it does matter to some degree which tires you are running.
Myself, running 255/60-15's for over 35 years and a couple different brands have always run 32 PSI all the way around and have gotten excellent tread wear and decent handling.
Perhaps around 30 PSI for best ride quality would be a good starting point.
2025 C3 ('68-'73) of the Year Finalist - Unmodified
I have a '79. Running Cooper Cobras, 255/60-15. Factory door sticker states: Cold Air Pressure/ 30lbs front - 35lbs rear.
For best fuel economy: 20lbs front - 26lbs rear. I run 28lbs all around and like the ride I'm getting.
I have also rebuilt the entire suspension which made a heck of difference in ride and handling. Good luck.
I have a '79. Running Cooper Cobras, 255/60-15. Factory door sticker states: Cold Air Pressure/ 30lbs front - 35lbs rear.
For best fuel economy: 20lbs front - 26lbs rear. I run 28lbs all around and like the ride I'm getting.
Depends on the tires used. But, 30 psi is a good place to start. Go no lower, unless you KNOW that the tires you have are capable of such lower pressure.
P.S. When radial tires first made it to Corvettes (mid-70's) the GM engineers mistakenly thought that wide tires should have less pressure and actually spec'd them for mid-20 psi levels. BIG MISTAKE!! Lots of tire failures from over-flexing the sidewalls.
The Owner's Manuals for those cars and some tire pressure sticker repro's still call out those low pressures. DO NOT DO SO.